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Modified iron-molybdate catalysts with various metal oxides by a mechanochemical method: enhanced formaldehydeyield in methanol partial oxidation

Xue Liu, Lingtao Kong, Shengtao Xu, Chaofan Liu, Fengyun Ma

《化学科学与工程前沿（英文）》 2021年 第15卷 第5期   页码 1099-1110 doi: 10.1007/s11705-020-2008-8

摘要： A mechanochemical method was employed to prepare modified iron molybdate catalysts with various metal salts as precursors. The physicochemical properties of the iron molybdate catalysts were characterized, and their performances in catalyzing the reaction from methanol to formaldehyde (HCHO) were evaluated. Iron molybdate catalysts doped with Co(NO ) ·6H O and Al(NO ) ·9H O resulted in high HCHO yields. Compared with a commercial catalyst, the HCHO yields in the reaction with the modified catalyst at an optimal Co/Mo molar ratio reached 97.37%. According to chemical state analysis, the formation of CoO and the efficient decrease in the MoO sublimation rate could be important factors enhancing the HCHO yield in reactions catalyzed with iron molybdate doped with different Co/Mo mole ratios.

关键词： iron molybdate catalyst     metal oxides     methanol to formaldehyde     Co/Mo ratio     formaldehyde yield    

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Catalytic activities and mechanism of formaldehyde oxidation over gold supported on MnO

Guanglong PANG,Donghui WANG,Yunhong ZHANG,Chunyan MA,Zhengping HAO

《环境科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 447-457 doi: 10.1007/s11783-015-0808-8

摘要： MnO microspheres with various surface structures were prepared using the hydrothermal method, and Au/MnO catalysts were synthesized using the sol-gel method. We obtained three MnO microspheres and Au/MnO samples: coherent solid spheres covered with wire-like nanostructures, solid spheres with nanosheets, and hierarchical hollow microspheres with nanoplatelets and nanorods. We investigated the properties and catalytic activities of formaldehyde oxidation at room temperature. Crystalline structures of MnO are the main factor affecting the catalytic activities of these samples, and γ-MnO shows high catalytic performance. The excellent redox properties are responsible for the catalytic ability of γ-MnO . The gold-supported interaction can change the redox properties of catalysts and accelerate surface oxygen species transition, which can account for the catalytic activity enhancement of Au/MnO . We also studied intermediate species. The dioxymethylene (DOM) and formate species formed on the catalyst surface were considered intermediates, and were ultimately transformed into hydrocarbonate and carbonate and then decomposed into CO . A proposed mechanism of formaldehyde oxidation over Au/MnO catalysts was also obtained.

关键词： MnO2 microspheres     Au/MnO2     formaldehyde oxidation     γ-MnO2    

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Synthesis of TiO2 nano-particles and their photocatalytic activity for formaldehyde and methyl orange

XIAO Xinyan, ZHANG Huiping, CHEN Huanqin, LIAO Dongliang

《化学科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 178-183 doi: 10.1007/s11705-007-0033-5

摘要： TiO nano-particles were synthesized by sol-gel technique and characterized by X-ray diffractometer (XRD) and transmission electron microscope (TEM). Their photocatalytic activities for formaldehyde (FA) and methyl orange (MO) degradation were tested using degradation rate (η) as an evaluation index. Based on the orthogonal test results, the optimal condition for TiO preparation was obtained. Results showed that particle sizes were in the range of 10 40 nm, and that prepared TiO had better photocatalytic activity than P25. A simplified model was developed to evaluate the apparent quantum efficiency (Φapp) of this photocatalytic reaction system.

关键词： prepared     photocatalytic activity     apparent     photocatalytic     orthogonal    

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PLANT DENSITY, IRRIGATION AND NITROGEN MANAGEMENT: THREE MAJOR PRACTICES IN CLOSING YIELD GAPS FOR AGRICULTURAL

《农业科学与工程前沿（英文）》 2021年 第8卷 第4期 doi: 10.15302/J-FASE -2020355

摘要：

Agriculture faces the dual challenges of food security and environmental sustainability. Here, we investigate current maize production at the field scale, analyze the yield gaps and impacting factors, and recommend measures for sustainably closing yield gaps. An experiment was conducted on a 3.9-ha maize seed production field in arid north-western China, managed with border and drip irrigation, respectively, in 2015 and 2016. The relative yield reached 70% in both years. However, drip irrigation saved 227 mm irrigation water during a drier growing season compared with traditional border irrigation, accounting for 44% of the maize evapotranspiration (ET). Yield variability under drip irrigation was 12.1%, lower than the 18.8% under border irrigation. Boundary line analysis indicates that a relative yield increase of 8% to 10% might be obtained by optimizing the yield-limiting factors. Plant density and soil available water content and available nitrogen were the three major factors involved. In conclusion, closing yield gaps with agricultural sustainability may be realized by optimizing agronomic, irrigation and fertilizer management, using water-saving irrigation methods and using site-specific management.

 

关键词： boundary line analysis     irrigation method     precision agriculture     spatial variability     yield gaps     yield-limiting factors    

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The effect of conservation tillage on crop yield in China

Hongwen LI,Jin HE,Huanwen GAO,Ying CHEN,Zhiqiang ZHANG

《农业科学与工程前沿（英文）》 2015年 第2卷 第2期   页码 179-185 doi: 10.15302/J-FASE-2015058

摘要： Traditional agricultural practices have resulted in decreased soil fertility, shortage of water resources and deterioration of agricultural ecological environment, which are seriously affecting grain production. Conservation tillage (CT) research has been developed and applied in China since the 1960s and 1970s, and a series of development policies have been issued by the Chinese government. Recent research and application have shown that CT has positive effects on crop yields in China. According to the data from the Conservation Tillage Research Center (CTRC), Chinese Ministry of Agriculture (MOA), the mean crop yield increase can be at least 4% in double cropping systems in the North China Plain and 6% in single cropping systems in the dryland areas of North-east and North-west China. Crop yield increase was particularly significant in dryland areas and drought years. The mechanism for the yield increase in CT system can be attributed to enhanced soil water content and improved soil properties. Development strategies have been implemented to accelerate the adoption of CT in China.

关键词： conservation tillage     crop yield     soil structure     development strategies    

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Breeding strategies for increasing yield potential in super hybrid rice

Shihua CHENG,Xiaodeng ZHAN,Liyong CAO

《农业科学与工程前沿（英文）》 2015年 第2卷 第4期   页码 277-282 doi: 10.15302/J-FASE-2015081

摘要： Super hybrid rice breeding is a new breeding method combining semi-dwarf breeding and heterosis breeding using germplasm and gene-environment interactions. This paper reviews the breeding strategies of super hybrid rice breeding in China, focusing on the utilization of heterosis of indica and japonica subspecies, construction of ideal plant architecture and pyramiding of disease resistant genes in restorer lines. To develop super hybrid rice, considerable effort should be made to explore genes related with high yield, good quality, resistance to pests and diseases, tolerance to stresses. Molecular breeding methods in combination with crossing techniques should be adopted in super hybrid rice breeding.

关键词： super hybrid rice     breeding strategies     yield potential    

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Highlight yield forming and innovative technologies in tropical crops

Wenquan WANG

《农业科学与工程前沿（英文）》 2016年 第3卷 第4期   页码 283-284 doi: 10.15302/J-FASE-2016128

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YIELD AND FRUIT QUALITY OF ALMOND, PEACH AND PLUM UNDER REGULATED DEFICIT IRRIGATION

《农业科学与工程前沿（英文）》 2021年 第8卷 第4期   页码 583-593 doi: 10.15302/J-FASE -2020325

摘要：

The effects of regulated deficit irrigation (RDI) on the performance of almond cv. Tuono, peach cv. JH-Hall and plum cv. Stanley were assessed on the Saiss Plain (NW, Morocco) over three consecutive growing seasons (2011–2013). Irrigation treatments consisted of a control, irrigation applied to fully satisfy crop water requirements (100% ETC), and two RDI treatments, irrigation applied to 75% ETC (RDI-75) and 50% ETC (RDI-50). These three treatments were applied during fruit-growth slowdown periods corresponding to Stages II and III in almond and Stage II in peach and plum. Yield and fruit quality traits were determined. The effect of RDI differed between species. Yield and fruit size were reduced significantly only in peach under RDI-50. Fruit quality improved in this species in the first year of the experiment, with an increase of sugar/acid ratio and polyphenol content. Plum quality also improved but the effects were significant only in the second and third years. Similar results were recorded in almond kernel, but their epidermal grooves were deeper under RDI-50, and this may have affected their commercial value. It is concluded that water can be saved during the fruit-growth slowdown period by up to 25% in peach and 50% in almond and plum with improvements in fruit quality without affecting total yield.

 

关键词： fruit quality / fruit yield / Prunus domestica / Prunus dulcis / Prunus persica / regulated deficit irrigation    

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Estimating the effect of urease inhibitor on rice yield based on NDVI at key growth stages

Kailou LIU,Yazhen LI,Huiwen HU

《农业科学与工程前沿（英文）》 2014年 第1卷 第2期   页码 150-157 doi: 10.15302/J-FASE-2014028

摘要： The effect of the urease inhibitor, N-(n-butyl) thiophosphoric triamide (NBPT) at a range of application rates on rice production was examined in a field experiment at Jinxian County, Jiangxi Province, China. The normalized difference vegetation index (NDVI) was measured at key growth stages in both early and late rice. The results showed that the grain yield increased significantly when urea was applied with NBPT, with the highest yield observed at 1.00% NBPT (wt/wt). NDVI differed with the growth stage of rice; it remained steady from the heading to the filling stage. Rice yield could be predicted from the NDVI taken at key rice growing stages, with ranging from 0.34 to 0.69 in early rice and 0.49 to 0.70 in late rice. The validation test showed that RMSE (t·hm ) values were 0.77 and 0.87 in early and late rice, respectively. Therefore, it was feasible to estimate rice yield for different amounts of urease inhibitor using NDVI.

关键词： normalized difference vegetation index (NDVI)     N-(n-butyl) thiophosphoric triamide (NBPT)     rice     grain yield    

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Lodging resistance and yield potential of winter wheat: effect of planting density and genotype

Yonggui XIAO,Jianjun LIU,Haosheng LI,Xinyou CAO,Xianchun XIA,Zhonghu HE

《农业科学与工程前沿（英文）》 2015年 第2卷 第2期   页码 168-178 doi: 10.15302/J-FASE-2015061

摘要： Improved lodging resistance is important for achieving high yield in irrigated environments. This study was conducted to determine genotypic variation in lodging resistance and related morphological traits among winter wheat cultivars planted at two densities, and to identify key traits associated with lodging resistance. Lodging performance of 28 genotypes, including 24 released cultivars and four advanced lines, was evaluated at 250 plants per square meter and 500 plants per square meter in Shandong province during the 2008–2009 and 2009–2010 crop seasons. At the higher density, the average grain yield was 2.6% higher, even though lodging score rose by as much as 136%. The higher planting density increased lodging through increased leaf area index (LAI), plant height, center of gravity and length of basal internodes, and reduced grain weight per spike and diameter of the lower two stem internodes. LAI, center of gravity and diameter of first internodes, as the important indicators for lodging resistance, were significantly correlated with lodging score, with = 0.62, 0.59 and −0.52 ( <0.01), respectively. Plant pushing resistance was significantly associated with diameter and length of the first internodes ( = 0.71–0.77, <0.01), indicating it could be used to assess the strength of the lower stem. Higher planting density could be used to select genotypes with lodging resistance in irrigated environments. Cultivars carrying high plant density tolerance and high yield potential, such as Jimai 22 and Liangxing 66, were recommended as leading cultivars for production as well as elite crossing parents for further increasing yield potential in the Yellow and Huai Valleys Winter Wheat Zone in China.

关键词： common wheat     yield potential     lodging performance     pushing resistance     leaf area index    

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Relationship between the number of tapping-induced secondary laticifer lines and rubber yield among

Yueyi CHEN,Xinsheng GAO,Xiaofei ZHANG,Weimin TIAN

《农业科学与工程前沿（英文）》 2016年 第3卷 第4期   页码 363-367 doi: 10.15302/J-FASE-2016122

摘要： The lack of suitable early selection parameters means that traditional rubber breeding for yield is time-consuming and inefficient. Laticifer is a tissue specific for natural rubber biosynthesis and storage in rubber tree. The number of the secondary laticifers in the trunk bark tissues is positively correlated with rubber yield in the matured rubber trees that are regularly tapped. In the present study, the rubber yield from 280 of 4–5 year-old virgin trees from 7 cross combinations was compared with the number of newly differentiated secondary laticifers caused by tapping. Results showed that the number of tapping-induced lines of secondary laticifers varied in different germplasm and was positively related to the rubber yield, indicating this could be used as a suitable parameter for early evaluation of yield potential of rubber trees.

关键词： Hevea brasiliensis     rubber yield breeding     early evaluation     tapping     secondary laticifer differentiation    

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PLANT DENSITY, IRRIGATION AND NITROGEN MANAGEMENT: THREE MAJOR PRACTICES IN CLOSING YIELD GAPS FOR AGRICULTURAL

Xiuwei GUO, Manoj Kumar SHUKLA, Di WU, Shichao CHEN, Donghao LI, Taisheng DU

《农业科学与工程前沿（英文）》 2021年 第8卷 第4期   页码 525-544 doi: 10.15302/J-FASE-2020355

摘要： Agriculture faces the dual challenges of food security and environmental sustainability. Here, we investigate current maize production at the field scale, analyze the yield gaps and impacting factors, and recommend measures for sustainably closing yield gaps. An experiment was conducted on a 3.9-ha maize seed production field in arid north-west China, managed with border and drip irrigation, respectively, in 2015 and 2016. The relative yield reached 70% in both years. However, drip irrigation saved 227 mm irrigation water during a drier growing season compared with traditional border irrigation, accounting for 44% of the maize evapotranspiration (ET). Yield variability under drip irrigation was 12.1%, lower than the 18.8% under border irrigation. Boundary line analysis indicates that a relative yield increase of 8% to 10% might be obtained by optimizing the yield-limiting factors. Plant density and soil available water content and available nitrogen were the three major factors involved. In conclusion, closing yield gaps with agricultural sustainability may be realized by optimizing agronomic, irrigation and fertilizer management, using water-saving irrigation methods and using site-specific management.

关键词： boundary line analysis     irrigation method     precision agriculture     spatial variability     yield gaps     yield-limiting factors    

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Genomics approaches to unlock the high yield potential of cassava, a tropical model plant

Shengkui ZHANG,Ping’an MA,Haiyan WANG,Cheng LU,Xin CHEN,Zhiqiang XIA,Meiling ZOU,Xinchen ZHOU,Wenquan WANG

《农业科学与工程前沿（英文）》 2014年 第1卷 第4期   页码 259-266 doi: 10.15302/J-FASE-2014043

摘要： Cassava, a tropical food, feed and biofuel crop, has great capacity for biomass accumulation and an extraordinary efficiency in water use and mineral nutrition, which makes it highly suitable as a model plant for tropical crops. However, the understanding of the metabolism and genomics of this important crop is limited. The recent breakthroughs in the genomics of cassava, including whole-genome sequencing and transcriptome analysis, as well as advances in the biology of photosynthesis, starch biosynthesis, adaptation to drought and high temperature, and resistance to virus and bacterial diseases, are reviewed here. Many of the new developments have come from comparative analyses between a wild ancestor and existing cultivars. Finally, the current challenges and future potential of cassava as a model plant are discussed.

关键词： cassava     genomics     yield potential     adaptability     tropical model    

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Electrorheological damper for the ultra-precision air bearing stage

ZHU Yu, JIA Songtao, CHEN Yaying, LI Guang

《机械工程前沿（英文）》 2008年 第3卷 第2期   页码 158-163 doi: 10.1007/s11465-008-0031-4

摘要： This paper illustrates how the electrorheological damper substantially improves the performance of the ultra-precision air bearing stage. Smart materials such as electrorheological fluids have attracted many researchers’ attention because of their resistance changeable performance in different electric fields. Meanwhile, the ultra-precision air bearing stage driven by the linear-motor is characterized by zero mechanical damping and poor anti-disturbance. To solve this problem and consider the characteristics of electrorheological fluids, an electrorheological damper is proposed in this paper. The electrorheological damper’s characteristics in high electric fields are obtained based on the Eyring constitutive model, which smoothly transits from the pre-yield to post-yield region. To enhance the performance of the electrorheological damper, which takes effect only when the stage is going to decelerate or position, the on-off and sliding mode control methods design and optimize the controller. The results prove that by using the advanced sliding mode control method, the characteristics of the ultra-precision air bearing stage can be effectively improved through the introduction of the electrorheological damper.

关键词： post-yield     linear-motor     advanced sliding     pre-yield     position    

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HOW MULTISPECIES INTERCROP ADVANTAGE RESPONDS TO WATER STRESS: A YIELD-COMPONENT ECOLOGICAL FRAMEWORK

《农业科学与工程前沿（英文）》 2021年 第8卷 第3期   页码 416-431 doi: 10.15302/J-FASE-2021412

摘要：

Absolute yield and land use efficiency can be higher in multicrops. Though this phenomenon is common, it is not always the case. Also, these two benefits are frequently confused and do not necessarily occur together. Cropping choices become more complex when considering that multicrops are subject to strong spatial and temporal variation in average soil moisture, which will worsen with climate change. Intercropping in agroecosystems is expected to buffer this impact by favoring resistance to reduced humidity, but there are few empirical/experimental studies to validate this claim. It is not clear if relatively higher multicrop yield and land use efficiency will persist in the face of reduced soil moisture, and how the relation between these benefits might change. Here, we present a relatively simple framework for analyzing this situation. We propose a relative multicrop resistance (RMR) index that captures all possible scenarios of absolute and relative multicrop overyield under water stress. We dissect the ecological components of RMR to understand the relation between higher multicrop yield and land use efficiency and the ecological causes of different overyield scenarios. We demonstrate the use of this framework with data from a 128 microplot greenhouse experiment with small annual crops, arranged as seven-species multicrops and their corresponding monocrops, all under two contrasting watering regimes. We applied simple but robust statistical procedures to resulting data (based on bootstrap methods) to compare RMR, and its components, between different plants/plant parts. We also provide simple graphical tools to analyze the data.

 

关键词： agroecosystem sustainability     crop overyielding     intercrop drought resistance     overyield ecological components    

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标题 作者 时间 类型 操作

Modified iron-molybdate catalysts with various metal oxides by a mechanochemical method: enhanced formaldehydeyield in methanol partial oxidation

Xue Liu, Lingtao Kong, Shengtao Xu, Chaofan Liu, Fengyun Ma

期刊论文

Catalytic activities and mechanism of formaldehyde oxidation over gold supported on MnO

Guanglong PANG,Donghui WANG,Yunhong ZHANG,Chunyan MA,Zhengping HAO

期刊论文

Synthesis of TiO2 nano-particles and their photocatalytic activity for formaldehyde and methyl orange

XIAO Xinyan, ZHANG Huiping, CHEN Huanqin, LIAO Dongliang

期刊论文

PLANT DENSITY, IRRIGATION AND NITROGEN MANAGEMENT: THREE MAJOR PRACTICES IN CLOSING YIELD GAPS FOR AGRICULTURAL

期刊论文

The effect of conservation tillage on crop yield in China

Hongwen LI,Jin HE,Huanwen GAO,Ying CHEN,Zhiqiang ZHANG

期刊论文

Breeding strategies for increasing yield potential in super hybrid rice

Shihua CHENG,Xiaodeng ZHAN,Liyong CAO

期刊论文

Highlight yield forming and innovative technologies in tropical crops

Wenquan WANG

期刊论文

YIELD AND FRUIT QUALITY OF ALMOND, PEACH AND PLUM UNDER REGULATED DEFICIT IRRIGATION

期刊论文

Estimating the effect of urease inhibitor on rice yield based on NDVI at key growth stages

Kailou LIU,Yazhen LI,Huiwen HU

期刊论文

Lodging resistance and yield potential of winter wheat: effect of planting density and genotype

Yonggui XIAO,Jianjun LIU,Haosheng LI,Xinyou CAO,Xianchun XIA,Zhonghu HE

期刊论文

Relationship between the number of tapping-induced secondary laticifer lines and rubber yield among

Yueyi CHEN,Xinsheng GAO,Xiaofei ZHANG,Weimin TIAN

期刊论文

PLANT DENSITY, IRRIGATION AND NITROGEN MANAGEMENT: THREE MAJOR PRACTICES IN CLOSING YIELD GAPS FOR AGRICULTURAL

Xiuwei GUO, Manoj Kumar SHUKLA, Di WU, Shichao CHEN, Donghao LI, Taisheng DU

期刊论文

Genomics approaches to unlock the high yield potential of cassava, a tropical model plant

Shengkui ZHANG,Ping’an MA,Haiyan WANG,Cheng LU,Xin CHEN,Zhiqiang XIA,Meiling ZOU,Xinchen ZHOU,Wenquan WANG

期刊论文

Electrorheological damper for the ultra-precision air bearing stage

ZHU Yu, JIA Songtao, CHEN Yaying, LI Guang

期刊论文

HOW MULTISPECIES INTERCROP ADVANTAGE RESPONDS TO WATER STRESS: A YIELD-COMPONENT ECOLOGICAL FRAMEWORK

期刊论文